Abstract

A study is presented on the applicability of the distribution coefficient (K_d) absorption/desorption model to simulate dissolved ¹³⁷Cs concentrations in Fukushima river water. The upstream Ota River basin was simulated using GEneral-purpose Terrestrial Fluid-flow Simulator (GETFLOWS) for the period 1 January 2014 to 31 December 2015. Good agreement was obtained between the simulations and observations on water and suspended sediment fluxes, and on particulate bound ¹³⁷Cs concentrations under both base and high flow conditions. By contrast the measured concentrations of dissolved ¹³⁷Cs in the river water were much harder to reproduce with the simulations. By tuning the K_d values for large particles, it was possible to reproduce the mean dissolved ¹³⁷Cs concentrations during base flow periods (observation: 0.32 Bq/L, simulation: 0.36 Bq/L). However neither the seasonal variability in the base flow dissolved ¹³⁷Cs concentrations (0.14-0.53 Bq/L), nor the peaks in concentration that occurred during storms (0.18–0.88 Bq/L, mean: 0.55 Bq/L), could be reproduced with realistic simulation parameters. These discrepancies may be explained by microbial action and leaching from organic matter in forest litter providing an additional input of dissolved ¹³⁷Cs to rivers, particularly over summer, and limitations of the K_d absorption/desorption model. It is recommended that future studies investigate these issues in order to improve simulations of dissolved ¹³⁷Cs concentrations in Fukushima rivers.

K. Sakuma, H. Tsuji, S. Hayashi, H. Funaki, A. Malins, K. Yoshimura, H. Kurikami, A. Kitamura, K. Iijima, M. Hosomi
Journal of Environmental Radioactivity 184-185, 53-62 (2018)

DOI: 10.1016/j.jenvrad.2018.01.001
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